Comprehensive overview of polyoxometalates for electrocatalytic hydrogen evolution reaction

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作者: Zonish Zeb Yichao Huang Lulu Chen Wenbo Zhou Meihong Liao Yangyang Jiang Haitao Li Limin Wang Lin Wang Hang Wang Tong Wei Dejin Zang Zhuangjun Fan Yongge Wei

作者单位: ³School of Mechanical and Electronic Engineering, Qingdao Binhai University, Qingdao, Shandong 266555, PR China ⁴Institute of Materia Medica, Shandong First Medical University & Shandong Academy of Medical Sciences, Jinan 250117, PR China ²State Key Laboratory of Heavy Oil Processing, School of Materials Science and Engineering, China University of Petroleum, Qingdao 266580, PR China ¹Key Lab of Organic Optoelectronics & Molecular Engineering of Ministry of Education, Department of Chemistry, Tsinghua University, Beijing 100084, PR China

关键词: Polyoxometalates Transition metals Electrocatalysts Hydrogen evolution reaction Water splitting

摘要: Electrocatalytic water splitting via hydrogen evolution reaction from renewable energy sources is an attractive alternative to produce hydrogen, but it still encounters the limitations of large-scale applicability of Pt-based electrocatalysts. Therefore, abundant efforts have been devoted to design and fabricate highly efficient and stable noble-metal-free electrocatalysts to replace the expensive Pt-based electrocatalysts. Recently, polyoxometalates and their derivatives have been proven to p...更多; Electrocatalytic water splitting via hydrogen evolution reaction from renewable energy sources is an attractive alternative to produce hydrogen, but it still encounters the limitations of large-scale applicability of Pt-based electrocatalysts. Therefore, abundant efforts have been devoted to design and fabricate highly efficient and stable noble-metal-free electrocatalysts to replace the expensive Pt-based electrocatalysts. Recently, polyoxometalates and their derivatives have been proven to provide plentiful opportunities for designing and fabricating highly efficient and stable noble-metal-free HER electrocatalysts with controllable catalytic active sites and well-defined nanostructures. In this review, recent advances on coordination structures and HER performances of POMs-contained composites and POMs-derived transition metal carbides, chalcogenides, phosphides, nitrides and other electrocatalysts have been discussed.收起

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